Wafer-scale synthesis of monolayer two-dimensional porphyrin polymers for hybrid superlattices

Yu Zhong; Baorui Cheng; Chibeom Park; Ariana Ray; Sarah Brown; Fauzia Mujid; Jae-Ung Lee; Hua Zhou; Joonki Suh; Kan-Heng Lee; Andrew J. Mannix; Kibum Kang; S. J. Sibener; David A. Muller; Jiwoong Park

doi:10.1126/science.aax9385

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Wafer-scale synthesis of monolayer two-dimensional porphyrin polymers for hybrid superlattices

View ORCID ProfileYu Zhong ¹,*,
View ORCID ProfileBaorui Cheng¹,*,
View ORCID ProfileChibeom Park¹,²,
View ORCID ProfileAriana Ray³,
View ORCID ProfileSarah Brown¹,²,
View ORCID ProfileFauzia Mujid ¹,
View ORCID ProfileJae-Ung Lee⁴,⁵,
View ORCID ProfileHua Zhou⁶,
Joonki Suh¹,
Kan-Heng Lee⁴,⁷,
View ORCID ProfileAndrew J. Mannix²,
View ORCID ProfileKibum Kang¹,²,⁸,
View ORCID ProfileS. J. Sibener ¹,²,
View ORCID ProfileDavid A. Muller ⁷,
View ORCID ProfileJiwoong Park ¹,²,⁴,†

¹Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.
²James Franck Institute, University of Chicago, Chicago, IL 60637, USA.
³Department of Physics, Cornell University, Ithaca, NY 14853, USA.
⁴Pritzker School of Molecular Engineering, University of Chicago, Chicago, IL 60637, USA.
⁵Department of Physics, Ajou University, Suwon 16499, Republic of Korea.
⁶Advanced Photon Source, Argonne National Laboratory, Lemont, IL 60439, USA.
⁷School of Applied and Engineering Physics, Cornell University, Ithaca, NY 14853, USA.
⁸Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology, Daejeon 34141, Republic of Korea.

↵†Corresponding author. Email: jwpark{at}uchicago.edu

↵* These authors contributed equally to this work.

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Science 13 Dec 2019:
Vol. 366, Issue 6471, pp. 1379-1384
DOI: 10.1126/science.aax9385

Yu Zhong

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

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Baorui Cheng

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

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Chibeom Park

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

2James Franck Institute, University of Chicago, Chicago, IL 60637, USA.

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Ariana Ray

3Department of Physics, Cornell University, Ithaca, NY 14853, USA.

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Sarah Brown

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

2James Franck Institute, University of Chicago, Chicago, IL 60637, USA.

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Fauzia Mujid

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

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Jae-Ung Lee

4Pritzker School of Molecular Engineering, University of Chicago, Chicago, IL 60637, USA.

5Department of Physics, Ajou University, Suwon 16499, Republic of Korea.

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Hua Zhou

6Advanced Photon Source, Argonne National Laboratory, Lemont, IL 60439, USA.

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Joonki Suh

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

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Kan-Heng Lee

4Pritzker School of Molecular Engineering, University of Chicago, Chicago, IL 60637, USA.

7School of Applied and Engineering Physics, Cornell University, Ithaca, NY 14853, USA.

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Andrew J. Mannix

2James Franck Institute, University of Chicago, Chicago, IL 60637, USA.

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Kibum Kang

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

2James Franck Institute, University of Chicago, Chicago, IL 60637, USA.

8Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology, Daejeon 34141, Republic of Korea.

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S. J. Sibener

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

2James Franck Institute, University of Chicago, Chicago, IL 60637, USA.

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David A. Muller

7School of Applied and Engineering Physics, Cornell University, Ithaca, NY 14853, USA.

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Jiwoong Park

1Department of Chemistry, University of Chicago, Chicago, IL 60637, USA.

2James Franck Institute, University of Chicago, Chicago, IL 60637, USA.

4Pritzker School of Molecular Engineering, University of Chicago, Chicago, IL 60637, USA.

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For correspondence: jwpark@uchicago.edu

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